潘剑锋,刘启胜,卢青波,潘振华.催化微燃烧室内氢气和氧气预混合燃烧特性[J].农业机械学报,2016,47(2):357-363.
Pan Jianfeng,Liu Qisheng,Lu Qingbo,Pan Zhenhua.Combustion Characteristic of Premixed Hydrogen/Oxygen Mixture in Catalytic Micro-combustor[J].Transactions of the Chinese Society for Agricultural Machinery,2016,47(2):357-363.
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催化微燃烧室内氢气和氧气预混合燃烧特性   [下载全文]
Combustion Characteristic of Premixed Hydrogen/Oxygen Mixture in Catalytic Micro-combustor   [Download Pdf][in English]
投稿时间:2015-08-10  
DOI:10.6041/j.issn.1000-1298.2016.02.047
中文关键词:  微尺度燃烧  数值模拟  吹熄极限  表面反应  气相反应
基金项目:国家自然科学基金项目(51376082)、江苏省自然科学基金项目(BK20131253)和江苏省高校优势学科建设工程项目
作者单位
潘剑锋 江苏大学 
刘启胜 江苏大学 
卢青波 江苏大学 
潘振华 江苏大学 
中文摘要:针对带催化的微燃烧室内部氢氧预混合燃烧过程,利用CFD计算软件建立模型进行数值模拟,在实验验证的基础上改变入口参数,分析了表面反应与气相反应的相互作用以及催化反应对火焰吹熄极限的影响。结果表明,表面反应对气相反应中间产物的消耗会使气相反应强度减弱;在催化剂表面附近的反应以表面反应为主,在远离催化剂表面的反应以气相反应为主。催化剂的添加能够极大地拓宽火焰吹熄极限,在当量比为1.0时,催化燃烧室和无催化燃烧室的吹熄极限分别为46、22 m/s。在当量比为1.0时,表面反应强度最高,此时燃烧室出口截面温度最高。
Pan Jianfeng  Liu Qisheng  Lu Qingbo  Pan Zhenhua
Jiangsu University,Jiangsu University,Jiangsu University and Jiangsu University
Key Words:micro-scale combustion  numerical simulation  blow-off limit  surface reaction  gas-phase reaction
Abstract:The premixed hydrogen/oxygen combustion process in a catalytic micro-combustor was numerically simulated with CFD software. The interaction between gas-phase and catalytic reaction was analyzed by changing inlet parameters on the basis of experimental verification. Meanwhile, the blow-off limits for combustor with and without catalyst were also investigated. The results showed that gas-phase reaction was subdued with the intermediate products consumed in catalytic reaction. At the same velocity, the flame temperature of catalytic combustor was lower than that of non-catalytic combustor. The OH mass fraction near up-wall of Pt cell in catalytic combustion chamber was also lower than that near up-wall of SiC cell in non-catalytic combustor. While owing to the exothermic surface reaction with Pt cell, the temperature of Pt cell in catalytic combustor was higher than that of SiC cell in non-catalytic combustor. Catalytic reaction was dominant near the surface of catalyst, while gas-phase reaction was dominant away from the surface. The OH mass fraction distribution trend near the inner up-wall in catalytic combustor was consistent with that near the inner up-wall in non-catalytic combustor. The blow-off limit can be widened by adding catalyst. The blow-off limits for combustor with and without catalyst were 46 m/s and 22 m/s, respectively. At equivalence ratio of 1.0, the strongest activity of catalytic was shown, and the gas-phase reaction was obviously restrained. With the increase of equivalence ratio, the mean temperature of out-wall was risen at the beginning and then it was dropped later. The highest mean temperature of out-wall was achieved with equivalence ratio of 1.0.

Transactions of the Chinese Society for Agriculture Machinery (CSAM), in charged of China Association for Science and Technology (CAST), sponsored by CSAM and Chinese Academy of Agricultural Mechanization Science(CAAMS), started publication in 1957. It is the earliest interdisciplinary journal in Chinese which combines agricultural and engineering. It always closely grasps the development direction of agriculture engineering disciplines and the published papers represent the highest academic level of agriculture engineering in China. Currently, nearly 8,000 papers have been already published. There are around 3,000 papers contributed to the journal each year, but only around 600 of them will be accepted. Transactions of CSAM focuses on a wide range of agricultural machinery, irrigation, electronics, robotics, agro-products engineering, biological energy, agricultural structures and environment and more. Subjects in Transactions of the CSAM have been embodied by many internationally well-known index systems, such as: EI Compendex, CA, CSA, etc.

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